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You're probably thinking of Bach's Toccata and Fugue in D Minor; it's the one always played when decrepid castles are shown on-screen.
E. Power Biggs is the recognized Bach organ authority, and he has dozens of recordings out there.
Also, check into Walter/Wendy Carlos' "Switched-On Bach." The original in 1967 was the first commercial use of the Moog synthesizer as a dedicated musical instrument (not simple sound effects), and the revisited release in 2000 covers newer pieces.
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