Probably too late, but Simon Says is a fun one. Toddlers love to mimic their siblings.
Cardboard box. Trust me on this one. The little one will want to climb inside; with the older one, you can decorate the box.
Definitely second the fort notion; forts are always popular.
Random dance party. Put on some oldies and get down with your bad self.
Pots, pans, and wooden spoons spoons=impromptu band.
This thread is a goldmine!
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If I am not better, at least I am different. --Jean-Jacques Rousseau
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