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I dont know if it qualifies as a 'conversation' but the "you think i'm fucking funny" scene in Goodfellas is great!
Also "On the Waterfront" with Brando talking about how he could have been a "contender" is very powerful
Apocalypse Now is a very quotable movie but it all seems to be in the monologue (sp?) by Willard, Kilgore's surfing bit or Kurtz's speech at the end, rather than as a conversation.
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