You could try the Gothic rpgs for the PC. They are about as open ended as the Elder Scrolls games meaning they have a main storyline but you are free to pretty much ignore it if you wish and still find plenty of things to keep you occupied for quite a long time. They are also a bit more 'adult' than the Elder Scrolls series.
Another one to check out would be S.T.A.L.K.E.R. . Though more of an FPS than straight up RPG it offers a rich story and you are free to go almost anywhere anytime you want though there are some areas of the Zone that will eat you alive if you are not properly prepped to be there.
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