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Prince - Purple Rain
Can - She Brings the Rain
Nick Drake - Pink Moon
Pink Floyd - Great Gig in the Sky
Jimi Hendrix - The Wind Cries Mary
Clint Mansell - Lux Aeterna
Leonard Cohen - Suzanne
Charles Mingus - Better Git Hit in Your Soul
Dusty Springfield - Son of a Preacher Man
Ray Charles - Georgia on my Mind
Dick Dale - Surf Rider
I'll second Jeff Buckley's Hallelujah, that song gives me chills.
I know it's subjective, but my idea of a perfect song is one that is so well-crafted or captures a mood so perfectly that you would be hard pressed to improve on it in any way.
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