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Two evil charaters that will always stick with their actors no matter what other role they play are Buffalo Bill from Silence of the Lambs, and Private Pyle from Full Metal Jacket.
I cannot watch Ted Levine or D'Onofrio in any other show without seeing those characters.
And I know Pyle wasn't technically evil, but watching him transform over the first half of the film from a harmless simpleton to a hate filled timebomb waiting to explode was chilling. And it doesn't help that D'Onofrio has played several lowlifes in his career.
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