Great Teacher Onizuka has some great intro music--"Driver's High" by L'arc un Ciel. It's funny because it's mostly a rock song all in Japanese, but like typical J-pop the chorus features some English phrases.
I have to agree with everyone who's mentioned the music from Cowboy Bebop. Definitely some of my favorite stuff.
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If I am not better, at least I am different. --Jean-Jacques Rousseau
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