Like default said, there isn't any support for PS games on PSP (besides remakes onto UMD format, of course.) However, I wouldn't rule out the possibilty of emulators being made to work on the PSP. As we speak, there is a group of people trying to get a simple Linux running on Nintendo DS, so you never know what will happen 
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"And, isn't sanity really just a one-trick pony anyway? I mean all you get is one trick, rational thinking, but when you're good and crazy, oooh, oooh, oooh, the sky is the limit."
- The Tick
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