2001 for me, although it was hard to select just one. HAL and the early humanoid tossing the bone in the air were the best.
Clockwork would run a very close second. I loved the language in that film.
Full Metal Jacket - just for the first half of the movie alone. Vincent D'Onofrio was realistically scary as Pvt. Pyle, and R Lee Ermey as the DI did more than enough to scare off a large number of recruits for the Marines.
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