First of all, you need to start doing lower body. What's the point of having big arms if you've got twigs for legs? Your body will be out of proportion and won't look right. Try squats and leg presses for your quads, leg curls or straight-leg deadlifts for your hamstrings, and either standing or seated calf raises for your calves.
If you're wanting to put mass on your shoulders then you should also include some barbell or dumbbell shoulder presses in your routine, and perhaps some lateral raises. However, I would split that stuff up and not do it 3 times a week, your muscles need more time to rest than you're giving them, unless you're not working them hard enough which I'm guessing is the case. Don't finish a set just because you've reached a certain number, keep going until you can't lift anymore. So you should probably seperate your workouts by different muscle groups and only work them either once or twice a week. You're also missing back and tricep exercises. You've got a lot of work to do.
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