Lots of good ones.
There's a great one in <i>The Vanishing Tower</i> but It's a jawbreaker. Voilodion Ghagnasdiak. An there are plenty more in the Elric Books. Arioch, the Knight of Swords, Pyaray, and Theleb K'aarna, to name a couple.
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Originally posted by absorbentishe
Boris Baddenoff(SP?)
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Boris Badenov. He was at the top of my list. (Along with Keyser Soze, who many other folks mentioned.)
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Originally posted by PredeconInferno
Dmitri Ravinoff (Raven)
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A sovreign entity unto himself, the Raven is absolutely one of the coolest villians every, and definitely in the running for badass king of the literary world, but the name isn't particularly cool, at least, compared to the rest of the character, which is exceedingly cool.
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Originally posted by MPower
The tick had some great ones...
The Red Scare
Chainsaw Vigilante
The Tick (Bruce)
Man-eating Cow
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Let's not forget:
The Evil Midnight Bomber what Bombs at Midnight!, Proto Clown, Pineapple Pokopo, Octo Paganini and the Forte Brothers, and El Seed!
The Other Tick's name was Barry.
Chairface Chippendale has got to be the best of them, though.