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Too many to choose from but here are a few:
OP: Neon Genesis, Trigun, Cowboy Bebop, Kenshin, Lain, Boogiepop Phantom, Hellsing, Berserk
ED: Neon Genesis, Kenshin, Boogiepop Phantom, Ghost in the Shell: Stand Alone Complex
Of course, Hellsing, Rahxephon, Cowboy Bebop and a few others have great music through the entire series.
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