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Jimi Hendrix - Voodoo Chile (Slight Return)
This is a tough one.
There are a ton of really good songs out there... quite a few of my favorites have already been mentioned. A few of my favorites are probably more considered blues than rock.
That said - I'm going to go ahead and say that Hendrix's "Voodoo Chile" is the best rock song of all time not already mentioned.
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"The power of accurate observation is frequently called cynicism by those who don't have it." - George Bernard Shaw
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