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hah i read the title and was about to post FLCL as well... that show really is something, I love those gainax dudes...
at the risk of getting attacked for shoujo, Kare Kano is very good, and by the same studio that did FLCL so you know there's some experimental animation involved.. good show, id be careful about who i recommend it to, though. it's excellent for what it is.
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