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The darkest classical music i know is also my favourite single piece of music in existance.
Henryk Gorecki- Symphony #3
But, if you mean "dark" as in "frightening and angry" check out any of the Omen soundtracks, composed by Jerry Goldsmith, preferably the first one. This is, hands down, the scariest music ever composed, and it's nice and "old" (unlike all the new movie scores now-a-days that all sound exactly alike. this music is truely unique)
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